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it's hard to say, since all those places SHOULD give the same chance of giving famed. But in that case, the place where you can kill most decent level enemies in the least time would be best (faster kill =more loot = more chance of skulls = more chance of famed), in other words, try the old cave in raven cove, where 4 ghosts stand in a straight line, use a buss with take aim and the most powerful ammo (try maxing steel shot + max take aim) and you should be able to take out 3 at a time.
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